Seems like a good idea to me. Am I right to think the number of PLLs with 4 edges bad is equal to the number of PLLs with 4 edges good? If so, memorizing twice the number of PLLs is not too bad.
Yup its the same number, but don't forget ... if you use this then there are some OLLs which you may as well forget
Not forget, just learn new algs for.
And what I said is only strictly true because this OLL has the same symmetries as OLL solved (full symmetry

).
Hmm, are you sure? I was thinking that
theoretically, you only need to know about 1/2 of your OLL's if you're using NEOPLL. You certainly don't need any of the no-edge flipped cases, because you can just use OCLLs for them.
For cases with two flipped edges, it seems like only half the number need to be known. For example imagine sune with a vertical bar:
Well if you know that, then you don't need to know this:
because applying an alg for the first case on the second one will give you an all-edge flip OLL. The same story is true of all the 'bar' cases.
Similarly, take this adjacent edge-flip sune:
And this one.
Applying the alg for one of these cases to the other gives an all-edge flip case, meaning you only need to know the alg for one of these two cases. And similarly for all (I think) adjacent edge flip OLLs.
The only set which you need to know all algs for is the all-corners oriented OLLs, and one of them is a NEOPLL OLL-skip!
If this is indeed the case, then it means that using NEOPLL+PLL can involve
less algs than straight OLL/PLL
